Ahhh.........if you come late to the party....all your choices are taken, BUT....
James Cagney - One,Two,Three; White Heat (incredible performance), Public Enemy
Edward G. Robinson - Our Vines Have Tender Grapes, The Stranger, Little Caesar
Humphrey Bogart - Casablanca, African Queen, Dead Reckoning
These are favorites and I just chose three for each....otherwise of course The Ten Commandments for EGR, Love Me or Leave Me and Never Steal Anything Small for JC, and The Barefoot Contessa and We're No Angels for HB.